The couple arrived in the capital city on Thursday, and were greeted by Ms Márquez and her husband, Rafael Yerney Pinillo.
Harry and Meghan in Colombia
The visit to the South American country, which has many similarities to the programme of an official royal overseas visit, is Prince Harry and Meghan's second this year after their three-day visit to Nigeria at the invitation of the West African nation's chief of defence staff.
Take a look at HELLO!'s favourite pictures from the tour...
1/10
On a roll
The Duke and Duchess appeared in high spirits on day three as they learnt new drumming skills from the Escuela Taller Tambores de Cabildo de la Boquilla - a local drum school that preserves the artform of traditional African drumming.
2/10
Beat of the Drum
The couple looked very much in sync as they played on the drums.
3/10
Eyes for you
The Duke and Duchess kicked off their final day by attending a panel discussion titled "Afro Women and Power" Forum at Valle del Cauca, the Municipal Theater in Cali - and the pair couldn't take their eyes off each other.
4/10
All smiles
The Duke and Duchess of Sussex radiated gorgeous smiles when they headed to San Basilio de Palenque.
5/10
Smitten selfie
Meghan and Harry were all smiles as they posed for a sweet selfie during their visit to the Centro de Rehabilitación Inclusiva.
6/10
Hand in hand
At a press conference ahead of Harry and Meghan's arrival, Ms Marquez described the Sussexes' trip as a "very special visit" aimed at building bridges and joining forces against cyber-bullying. Here, the couple made a very stylish entrance to kick off the visit.
7/10
Sweet exchange
The Sussexes spent a relaxed afternoon at the vice president's residence, exchanging gifts and enjoying traditional Colombian hospitality.
8/10
A warm welcome
The Sussexes spent a relaxed afternoon at the vice president's residence, exchanging gifts and enjoying traditional Colombian hospitality. Later, Harry and Meghan attended a folkloric presentation at Centro Nacional de las Artes Delia Zapata.
9/10
Just the two of them
There was also a sweet PDA moment between the Sussexes as Meghan leaned into her husband and Harry kissed the top of her head.
10/10
Deep in conversation
The Duke and Duchess took time to greet and applaud all of the performers, dancers, actors, and crew who were involved with the day’s programming.
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